No, it is not possible to link an existing Cryptocurrency Service Provider account to an IBKR account. If you want a Cryptocurrency Service Provider account linked to your IBKR account then you will need to request cryptocurrency trading permissions in your IBKR securities brokerage account, at which point a new Cryptocurrency Service Provider account will be created for you and linked to your IBKR trading platform's interface.
Additional Information
All exchange and custody services in connection with trading and holding cryptocurrency tokens and other digital asset tokens through IBKR trading platforms are provided by Cryptocurrency Service Providers. Learn more.